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This book describes various carbon nanomaterials and their unique properties, and offers a detailed introduction to graphene-carbon nanotube (CNT) hybrids. It demonstrates strategies for the hybridization of CNTs with graphene, which fully utilize the synergistic effect between graphene and CNTs. It also presents a wide range of applications of graphene-CNT hybrids as novel materials for energy storage and environmental remediation. Further, it discusses the preparation, structures and properties of graphene-CNT hybrids, providing interesting examples of three types of graphene-CNT hybrids with different nanostructures. This book is of interest to a wide readership in various fields of materials science and engineering.